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Nanomaterials 2023, 13, x FOR PEER REVIEW 10 of 22 Nanomaterials 2023, 13, 1257 9 of 20 Materials Electrolyte Specific Capaci- tance 20 M 1-butyl-3- methylim- 480 F g+1 at 20 mV Energy Den- sity 110 Whkg−1 Power Density 10 kWkg−1 Cyclic Stability Ref. 2.56% capacitance loss after500cycles [94] Figure 4. (a) Photograph of the corresponding components of a hybrid DES. (b) A plot illustrating Figure 4. (a) Photograph of the corresponding components of a hybrid DES. (b) A plot illustrating the changes in ionic conductivity of DES electrolytes with varying molar ratios of acetonitrile/water the changes in ionic conductivity of DES electrolytes with varying molar ratios of acetonitrile/water mixtures. Reprinted with the permission of [90]. (c) MD simulation of a DES system prepared from mixtures. Reprinted with the permission of [90]. (c) MD simulation of a DES system prepared from the the ternary mixture of choline chloride, ethylene glycol, and urea. Reprinted with the permission of t[e9r1n]a.ry mixture of choline chloride, ethylene glycol, and urea. Reprinted with the permission of [91]. 4. Supercapacitor Performance of Two-Dimensional (2D) Electrode Material in Novel 4. Supercapacitor Performance of Two-Dimensional (2D) Electrode Material in Novel Aqueous Electrolytes Aqueous Electrolytes Two-dimensional materials are promising electrodes for supercapacitors because of Two-dimensional materials are promising electrodes for supercapacitors because of their excellent capacitive performances, high energy, long cycle life, and power density. their excellent capacitive performances, high energy, long cycle life, and power density. MXenes, graphene materials, metal oxides, metal nitrides, metal sulfides, and metal–organic MXenes, graphene materials, metal oxides, metal nitrides, metal sulfides, and metal– frameworks are some examples of 2D materials [93]. The porous structure, surface area, and organic frameworks are some examples of 2D materials [93]. The porous structure, sur- capability for ion intercalation are some factors contributing to the improved performance face area, and capability for ion intercalation are some factors contributing to the im- of 2D electrode materials. Recently, supercapacitors made from the combination of 2D proved performance of 2D electrode materials. Recently, supercapacitors made from the electrode materials with nonconventional electrolytes have attracted special concern due to graphene nanoplate- lets-coatedcarbonpaper idazoliumchloride+0.1M s−1 combination of 2D electrode materials with nonconventional electrolytes have attracted their high performance. Table 1 compares the electrochemical performances of a few 2D special concern due to their high performance. Table 1 compares the electrochemical layered materials with different WIS/DES electrolyte systems. performances of a few 2D layered materials with different WIS/DES electrolyte systems. Table 1. A summary of the performance of 2D electrode materials in nonconventional electrolytes. 4-hydroxy-2,2,6,6-tetramethPDF Image | Water-in-Salt Eutectic Solvent-Based Liquid Electrolytes
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