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seeking to mitigate the rate of this degradation, specifically through use of electrochemical purification of the electrolyte to remove common metal impurities that catalyze the side reaction. This study brings the Fe-Cr chemistry one step closer to being commercially viable. In summary, the goal of my thesis is to help close the gap between the existing, predominantly lab-based understanding of RFBs and the understanding needed for successful, long-term, and competitive grid-scale implementation of RFBs. Greater demand for grid-scale RFBs is being held back by concerns around their high prices and perceived risk. While many researchers working on RFBs are exploring exciting new materials, chemistries, architectures, etc., some concerted effort to increase the RFB’s TRL, such that it can be reliably deployed, would go a long way to boost its appeal to investors. Unlike the more-developed, incumbent lithium-ion technology, the RFB field neither has the time – as deadlines to decarbonize the grid to prevent irreversible climate change are rapidly approaching – nor the alternative beachhead markets to slowly develop a commercially viable RFB solution that can economically compete on the grid. The RFB industry will strongly benefit from more upfront due diligence, via methods like techno-economic modeling, to solve practical questions and design technically and economically feasible systems. My research has developed new techno-economic models that better describe RFB costs, performance, degradation, and maintenance, and further used these models to determine paths for new research and development that provide the best economic returns and, in turn, drive RFB deployment. 15PDF Image | Bringing Redox Flow Batteries to the Grid
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