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5 Single fibre electrode measurements - a versatile strategy for assessing the non-uniform kinetics Discrepancies between the simulated and experimental cyclic voltammograms can be seen in the non-peak regions in Figure 5.4c, even after both the void size distribution and rate constant distribution have been considered. This is likely due to the electrode capacitance, which is not included in the model. The fraction of capacitive current relative to the faradaic current from the redox reaction increases as the sweep rate increases. Because of this, there is poorer agreement between the simulated and measured voltammograms in the non-faradaic regions as the sweep rate increases. The presence of capacitance has also been shown to alter the peak separation, voltammogram shape and peak current at planar electrodes, particularly at faster sweep rates and this likely contributes to the discrepancies observed in (Figure 5.4c) [190]. 64PDF Image | Electron Transfer Kinetics in Redox Flow Batteries
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