Organic Redox Flow Batteries 2023

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Organic Redox Flow Batteries 2023 ( organic-redox-flow-batteries-2023 )

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Figure 3.1: (Left) Current-overpotential curves simulated from Equation 3.7, using i0 = 1 mA cm−2, n = 1, T = 298.15 K, and α as indicated in the legends. (Right) Absolute values of the current densities shown to the left on a logarithmic scale. are shown in Figure 3.2. Note that the potential is reported versus the standard hydrogen electrode (SHE), which will be the reference of choice for presenting voltammograms for the remainder of this work. Figure 3.2: (Left) Potential-time profile during a CV experiment. (Right) Typical cyclic voltammogram of a reversible system with annotations of the peak and half-wave potentials (blue) and peak current densities (red). The current density is commonly reported instead of the current to ease comparison of voltammograms recorded on working electrodes with different geometric surface areas. CV is carried out in a three-electrode configuration, consisting of a working electrode (WE), counter electrode (CE), and reference electrode (RE), all immersed in an elec- trolyte. The electrochemical reaction under investigation takes place at the WE, which consists of a disk of conductive and inert material, such as glassy carbon, gold, or plat- inum, embedded in an insulating and inert material, typically a polymer. The CE is coupled with the WE to provide a circuit over which the current is applied or measured 3.2. Cyclic voltammetry 21

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