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8 9 Conclusions ..................................................................208 Appendix ......................................................................213 10 9.1 9.1.1 One step, one-electron process..................................................213 Kinetics of redox reactions................................................................213 9.1.2 Implications of Butler-Volmer model for the one-step, one-electron process 216 9.1.2.1 Equilibrium conditions. The exchange current ........................216 9.1.2.2 The current-overpotential equation....................................... 217 9.1.2.3 Approximate Form of the i-η Equation ..................................218 9.1.2.3.1 9.1.2.4 Effects of Mass Transfer ......................................................220 Tafel plots ......................................................................218 9.1.3 Multistep mechanisms...............................................................223 9.1.3.1 Rate-determining electron transfer ....................................... 224 9.1.3.2 Multistep Process at Equilibrium ........................................... 225 9.1.3.3 Quasirreversible and Irreversible Multistep Processes ............. 227 9.2 Active surface area..........................................................................229 9.3 Transport phenomena ......................................................................230 9.3.1 Rotating disk electrode .............................................................231 9.3.1.1 Solution of the Convective-Diffusion Equation........................232 9.3.1.2 General Current-Potential Curves at the RDE.........................233 9.3.2 Electrolyte flow ........................................................................235 9.3.3 Reactant concentration effects...................................................238 References ...................................................................240PDF Image | Redox Flow Batteries Vanadium to Earth Quinones
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