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Batteries 2022, 8, x FOR PEER REVIEW 8 of 19 8 of 20 FiguFrigeu4re. 4In. IintiiatilalSSEII formaatitoionnanadntdhetmheodmelsoadfetelsr 1a0fcteyrcle1s0inctyhceleslecitnrotlhyte oefle(ac–trco) lNyatePFo6 fFE(aC––cf)reNe aPF6 FECE−Cfr:eDeMEC–:bDasMedCe−lbeactsreodlyetel,e(cdtr–of)lyNtea,P(Fd6–EfC):NDaMPCF6–bEaCse:dDeMleCct−roblaystedweitlhecFtEroClyatdedwitiivteh[4F4E]C;waidthditive [44]p;ewrmitihssipoenrfmroimssiSopnrinfrgoemrNSatpurrien,gceorpyNriagthutr2e0,21c.o(pgy)rPiVghdtFa2n0d21B.i(pgo)wPdVerd(FnaamnedPBBi@pCouw)–dceorat(endamed Batteries 2022, 8, 272 PB@Cuuf)o−icloaantdedthCeurefpoeial taenddNtaheplraetpinega/testdriNppainpglaptirnocge/sstreisp; p(hin) gthperfoclleoswseins;g(Nh)atphleatfionlglo/wstrinipgpiNnga plat- −2 −2 −2 −2 ing/tsetsrtipatpaincgurtresnttadtenascituyrorfen1tmdAencmsityoanfd1amreAaccampaciatynodfa2rmeaAchacpmacity[4o7]f.2RemprAohduccmedw[4it7h].thReepro- ducpedermwistshiotnheofprerf.m[4is7s]iEolnseovfierre,fc.o[p4y7r]igEhlste2v02ie2r., copyright 2022. Artificial SEI is an attractive solution to overcome the inherent shortcomings of the Artificial SEI is an attractive solution to overcome the inherent shortcomings of the SEI layer [48]. Since the artificial SEI is constructed outside the battery, the composition, SEI layer [48]. Since the artificial SEI is constructed outside the battery, the composition, thickness, and mechanical properties of the interphase can be precisely designed. Fur- thickness, and mechanical properties of the interphase can be precisely designed. Further- thermore, the morphology of the deposited sodium metal can be precisely controlled due more, the morphology of the deposited sodium metal can be precisely controlled due to to the tunable SEI layer [49,50]. According to the previous studies, the design of a stable theatrutinfiacbialleSSEEIIshlaoyueldrf[o4l9lo,5w0]t.hArececporidncinipgletso:(tih)eitpcarneveifofeucstivsteulydbielosc,kththeedresaicgtinonobfeatwsteaebnlear- tifictihael eSlEecItsrohloyuteldanfdolslodwiutmhrmeeetparl;in(ici)ipitlehsa:s(gi)oiotdcaioniecffceocntdivuecltyivbitlyo, cakllotwheinrgeasmctoionthbieotnween transportation including single ions; and (iii) it has good mechanical stability and can with- the electrolyte and sodium metal; (ii) it has good ionic conductivity, allowing smooth ion stand repeated deposition and stripping processes of the sodium metal. At present, various transportation including single ions; and (iii) it has good mechanical stability and can inorganic– or organic–based artificial SEI have been reported for sodium metal batteries, withstand repeated deposition and stripping processes of the sodium metal. At present, various inorganic− or organic−based artificial SEI have been reported for sodium metal batteries, including graphene [51], polyvinylidene fluoride (PVdF) [52], metal−organic framework materials [53], carbon nanotube paper [54], metal oxide layer, and some alloy- based artificial layers[55,56].PDF Image | Anode-Free Rechargeable Sodium-Metal Batteries
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