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Gels 2022, 8, 725 7 of 7 References Conflicts of Interest: The authors declare no conflict of interest. 1. Sun, C.; Liu, J.; Gong, Y.; Wilkinson, D.P.; Zhang, J. Recent advances in all-solid-state rechargeable lithium batteries. Nano Energy 2017, 33, 363–386. [CrossRef] 2. Choi, J.W.; Aurbach, D. Promise and reality of post-lithium-ion batteries with high energy densities. Nat. Rev. Mater. 2016, 1, 16013. [CrossRef] 3. Kulova, T.L.; Fateev, V.N.; Seregina, E.A.; Grigoriev, A.S. A brief review of post-lithium-ion batteries. Int. J. Electrochem. Sci. 2020, 15, 7242–7259. [CrossRef] 4. Ponrouch, A.; Bitenc, J.; Dominko, R.; Lindahl, N.; Johansson, P.; Palacín, M.R. Multivalent rechargeable batteries. Energy Storage Mater. 2019, 20, 253–262. [CrossRef] 5. Yang, J.; Zhang, H.; Zhou, Q.; Qu, H.; Dong, T.; Zhang, M.; Tang, B.; Zhang, J.; Cui, G. Safety-enhanced polymer electrolytes for sodium batteries: Recent progress and perspectives. ACS Appl. Mater. Interfaces 2019, 11, 17109–17127. [CrossRef] [PubMed] 6. Gebert, F.; Knott, J.; Gorkin III, R.; Chou, S.-L.; Dou, S.-X. Polymer electrolytes for sodium-ion batteries. Energy Storage Mater. 2021, 36, 10–30. [CrossRef] 7. Rakov, D.A.; Chen, F.; Ferdousi, S.A.; Li, H.; Pathirana, T.; Simonov, A.N.; Howlett, P.C.; Atkin, R.; Forsyth, M. Engineering high-energy-density sodium battery anodes for improved cycling with superconcentrated ionic-liquid electrolytes. Nat. Mater. 2020, 19, 1096–1101. [CrossRef] [PubMed] 8. Sun, J.; O’Dell, L.A.; Armand, M.; Howlett, P.C.; Forsyth, M. Anion-Derived Solid-Electrolyte Interphase Enables Long Life Na-Ion Batteries Using Superconcentrated Ionic Liquid Electrolytes. ACS Energy Lett. 2021, 6, 2481–2490. [CrossRef] 9. Hilder, M.; Howlett, P.C.; Saurel, D.; Gonzalo, E.; Armand, M.; Rojo, T.; Macfarlane, D.R.; Forsyth, M. Small quaternary alkyl phosphonium bis (fluorosulfonyl) imide ionic liquid electrolytes for sodium-ion batteries with P2-and O3-Na2/3 [Fe2/3Mn1/3] O2 cathode material. J. Power Sources 2017, 349, 45–51. [CrossRef] 10. Ferdousi, S.A.; O’Dell, L.A.; Sun, J.; Hora, Y.; Forsyth, M.; Howlett, P.C. High-Performance Cycling of Na Metal Anodes in Phosphonium and Pyrrolidinium Fluoro (sulfonyl) imide Based Ionic Liquid Electrolytes. ACS Appl. Mater. Interfaces 2022, 14, 15784–15798. [CrossRef] [PubMed] 11. Kalhoff, J.; Eshetu, G.G.; Bresser, D.; Passerini, S. Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives. ChemSusChem 2015, 8, 2154–2175. [CrossRef] [PubMed] 12. Fdz De Anastro, A.; Porcarelli, L.; Hilder, M.; Berlanga, C.; Galceran, M.; Howlett, P.; Forsyth, M.; Mecerreyes, D. UV-cross-linked ionogels for all-solid-state rechargeable sodium batteries. ACS Appl. Energy Mater. 2019, 2, 6960–6966. [CrossRef] 13. Chereddy, S.; Aguirre, J.; Dikin, D.; Wunder, S.L.; Chinnam, P.R. Gel electrolyte comprising solvate ionic liquid and methyl cellulose. ACS Appl. Energy Mater. 2019, 3, 279–289. [CrossRef] 14. Kido, R.; Ueno, K.; Iwata, K.; Kitazawa, Y.; Imaizumi, S.; Mandai, T.; Dokko, K.; Watanabe, M. Li+ ion transport in polymer electrolytes based on a glyme-Li salt solvate ionic liquid. Electrochim. Acta 2015, 175, 5–12. [CrossRef] 15. Hubble, D.; Qin, J.; Lin, F.; Murphy, I.A.; Jang, S.-H.; Yang, J.; Jen, A.K.-Y. Designing solvate ionogel electrolytes with very high room-temperature conductivity and lithium transference number. J. Mater. Chem. A 2018, 6, 24100–24106. [CrossRef] 16. Casas-Cabanas, M.; Roddatis, V.V.; Saurel, D.; Kubiak, P.; Carretero-González, J.; Palomares, V.; Serras, P.; Rojo, T. Crystal chemistry of Na insertion/deinsertion in FePO4–NaFePO4. J. Mater. Chem. 2012, 22, 17421–17423. [CrossRef] 17. Wongittharom, N.; Lee, T.-C.; Wang, C.-H.; Wang, Y.-C.; Chang, J.-K. Electrochemical performance of Na/NaFePO4 sodium-ion batteries with ionic liquid electrolytes. J. Mater. Chem. A 2014, 2, 5655–5661. [CrossRef] 18. Galceran, M.; Saurel, D.; Acebedo, B.; Roddatis, V.V.; Martin, E.; Rojo, T.; Casas-Cabanas, M. The mechanism of NaFePO4 (de) sodiation determined by in situ X-ray diffraction. Phys. Chem. Chem. Phys. 2014, 16, 8837–8842. [CrossRef] [PubMed] 19. Berlanga, C.; Monterrubio, I.; Armand, M.; Rojo, T.; Galceran, M.; Casas-Cabanas, M. Cost-effective synthesis of triphylite- NaFePO4 cathode: A zero-waste process. ACS Sustain. Chem. Eng. 2019, 8, 725–730. [CrossRef] 20. Saurel, D.; Giner, M.; Galceran, M.; Rodríguez-Carvajal, J.; Reynaud, M.; Casas-Cabanas, M. The triphylite NaFe1-yMnyPO4 solid solution (0≤ y≤ 1): Kinetic strain accommodation in NaxFe0.8 Mn0.2PO4. Electrochim. Acta 2022, 425, 140650. [CrossRef]PDF Image | Phosphonium Iongels for Solid-State Sodium Metal Batteries
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