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J. Phys. Energy 2 (2020) 032008 M Pasta et al batteries should be ideally suited to these applications, although several barriers to large-scale commercialisation currently exist. The overarching challenge is to improve our understanding of the processing-structure-properties relationships of thin-film cells, both at the materials and whole-cell levels. In terms of materials challenges, studying the ionic conduction mechanisms in amorphous electrolyte materials will aid the selection of appropriate candidates to succeed LiPON. Whole-cell challenges centre on internal cell interfaces and the need to maximise areal capacity without sacrificing power density. Relatively few investigations have been performed on 3D cell architectures; future studies must seek to achieve the optimum balance between cell performance and processability, and overcoming these challenges is likely to be the focus of thin-film cell research for the foreseeable future. Acknowledgments This work was supported by the Engineering and Physical Sciences Research Council [‘Enabling next generation lithium batteries’ EP/M009521/1] and the Faraday Institution [‘All-Solid-State Batteries with Li and Na Anodes’ FIRG007, FIRG008]. SJT acknowledges support from an EPSRC PhD studentship [project reference 2114670 related to EP/R513295/1]. 45PDF Image | 2020 roadmap on solid-state batteries
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