Next Generation Electrical Energy Storage

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Next Generation Electrical Energy Storage ( next-generation-electrical-energy-storage )

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Table of Contents Executive Summary...................................................................................................................................................................1 1 Introduction ...................................................................................................................................................................... 3 2 Priority Research Directions in Next Generation Electrical Energy Storage ........................................................ 7 2.1 PRD 1 — Tune Functionality of Materials and Chemistries to Enable Holistic Design for Energy Storage.................................................................................................................................................9 2.1.1 Scientific Challenges..................................................................................................................................................9 2.1.2 Research Thrusts........................................................................................................................................................14 2.1.3 References.................................................................................................................................................................. 20 2.2 PRD 2 — Link Complex Electronic, Electrochemical, and Physical Phenomena Across Time and Space ..................................................................................................................................... 23 2.2.1 Scientific Challenges ............................................................................................................................................... 24 2.2.2 Research Thrusts.......................................................................................................................................................27 2.2.3 References.................................................................................................................................................................. 35 2.3 PRD 3 — Control and Exploit the Complex Interphase Region Formed at Dynamic Interfaces ...........37 2.3.1 Scientific Challenges ............................................................................................................................................... 38 2.3.2 Research Thrusts.......................................................................................................................................................47 2.3.3 References................................................................................................................................................................... 51 2.4 PRD 4 — Revolutionize Energy Storage Performance through Innovative Assemblies of Matter ...... 55 2.4.1 Scientific Challenges...............................................................................................................................................55 2.4.2 Research Thrusts......................................................................................................................................................56 2.4.3 References.................................................................................................................................................................. 62 2.5 PRD 5 — Promote Self-healing and Eliminate Detrimental Chemistries to Extend Lifetime and Improve Safety............................................................................................................................................. 65 2.5.1 Scientific Challenges .............................................................................................................................................. 68 2.5.2 Research Thrusts......................................................................................................................................................69 2.5.4 References...................................................................................................................................................................75 3 Panel Reports for Next Generation Electrical Energy Storage ............................................................................. 77 3.1 Panel 1 Report — Pathways to Simultaneous High Energy and Power......................................................79 3.1.1 Current Status and Recent Advances.................................................................................................................79 3.1.2 Scientific Challenges and Opportunities .......................................................................................................... 82 3.1.3 Impact ........................................................................................................................................................................... 90 3.1.4 References.................................................................................................................................................................. 90 NEXT GENERATION ELECTRICAL ENERGY STORAGE iii

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