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5.4 Multi-stepmodel–validationattempts ................... 116 5.4.1 Ratecapability ............................. 117 5.4.2 Cyclicvoltammetry........................... 118 5.5 Multi-stepmodel–furthersimulations ................... 120 5.5.1 Galvanostatic charge/discharge profiles . . . . . . . . . . . . . . 120 5.5.2 Transport ................................ 121 5.5.3 Impedance................................ 125 5.5.4 Microstructure ............................. 128 5.6 Multi-stepmodel–polysulfideshuttleextension. . . . . . . . . . . . . . 129 5.7 Conclusions ................................... 132 5.7.1 Achievements.............................. 132 5.7.2 Shortcomings .............................. 133 5.7.3 Possibleimprovementsandoutlook................. 134 6 Conclusions and outlook 137 6.1 Summaryofachievements........................... 137 6.2 Limitationsofthisworkandideasforfutureresearch. . . . . . . . . . . 140 6.3 Outlookbeyondacademia........................... 141 A Appendix 143 A.1 Listofsymbols ................................. 143 A.2 Calculation of specific capacities, energy densities and state of charge . 146 A.3 Listofchemicals ................................ 148 A.4 Listofequipment................................ 149 A.5 Parametersetsforthemodels......................... 150 Bibliography 153 Citedpublications................................... 153 Ownpublications................................... 180 Academic résumé of David N. Fronczek 184 Acknowledgments 186 7PDF Image | Lithium-Sulfur Battery: Design, Characterization, and Physically-based Modeling
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