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Molecules 2019, 24, 182 2 of 41 Molecules 2019, 24, x FOR PEER REVIEW 2 of 42 polyurethanes, etc. [6] In the subsequent years, several short reviews describing special fields were also reviewed.Forexample,catalyticstrategyinsightsweregainedonthereactionofCO andaziridines and polyurethanes, etc. [6] In the subsequent years, several short reviews describing s2pecial fields (a10w0e%reaatlosmo recvoienwoemd.icFaolrreoxuatme)ptloe,pcaretaplyatriecostxrazteoglyidiinnsoignhetsawnedrepgoaliynuedreothnathnesreianc2ti0o1n2o[f1C2O]a2nandd2017 (hetearzoirgideineosu(as 1c0a0t%alyatsoismsecchoenmomesic)a[l1r3o]u. teS)utobsperqepuaernetolyxaiznol2id01in3o,nGeshaonsdh peotlyaul.resthuamnmesainri2z0e1d2 v[1a2r]ious and 2017 (heterogeneous catalysis schemes) [13]. Subsequently in 2013, Ghosh et al. summarized synthetic methods to produce oxazolidinones from CO2 with a variety of aziridines, propargylamines various synthetic methods to produce oxazolidinones from CO2 with a variety of aziridines, and 2-aminoalcohols [14]. In addition, part of a mini-review from the Tomishige group focuses propargylamines and 2-aminoalcohols [14]. In addition, part of a mini-review from the Tomishige on the direct conversion of CO2 with aminoalcohols and diamines to give cyclic carbamates and group focuses on the direct conversion of CO2 with aminoalcohols and diamines to give cyclic cyclic ureas via heterogeneous catalysts [15]. Recently, Li et al. focused on catalytic synthesis carbamates and cyclic ureas via heterogeneous catalysts [15]. Recently, Li et al. focused on catalytic of urea derivatives using CO2 and amines [16]. Moreover, a book chapter from the He group synthesis of urea derivatives using CO2 and amines [16]. Moreover, a book chapter from the He mainly focuses on the synthesis of carbonyl-containing chemicals, including 2-oxazolidinones and group mainly focuses on the synthesis of carbonyl-containing chemicals, including 2-oxazolidinones quinazoline-2,4(1H,3H)-diones, through C-N bond formation [17]. and quinazoline-2,4(1H,3H)-diones, through C-N bond formation [17]. Methodology research will provide a solid theory for CO2 conversion into value-added products Methodology research will provide a solid theory for CO2 conversion into value-added through C-N bond formation, and novel strategies have sprung up in the past few years. Herein, we products through C-N bond formation, and novel strategies have sprung up in the past few years. wouHlderleikine,twoehiwgholuilgdhtlirkecetnoth(2ig0h1l4ig–h2t01re8c)ednetv(e2l0o1p4m–2e0n18ts) idnecvaetloaplymtiecnmtseitnhocdatsaflyotrichmeemthicoadlsfifxoartion ofCcOhemtoicaflorfimxatvioanrioufsCcOh2emtoicfoarlsmthvraoruioguhsCch-eNmibcoalnsdthfroorumgahtiCon-N(Sbcohnedmfeor1m).atiNonot(aSbclhye,mthee1w).ork 2 descNriobteadblyin, theewporerkvidoeusscriebvediewinstwheilplrneovtiobuesdreisvcieuwssewdiilnl nthotisbreedvisecwu,ssuendleinssthspiserceiavlileywr,euqnuleirsesdin specially required in individual cases. individual cases. Scheme 1. CO2 conversion through C-N bond formation reactions described in this work. Scheme 1. CO2 conversion through C-N bond formation reactions described in this work. 2. C2h.eCmhiecmalicFailxFaitxioatnioonfoCfOCOt2hthrorouugghhC--NBondFormaattioionn 2 2.1. 2S.e1q.uSenqutieanltCiaalrCbaorxbyolxaytliaotnioannadndCCycylcilziaztaitoionnwiitthC-O/C-NBoonnddFForomrmataiotinon 2.1.1. Synthesis of Oxazolidinone Derivatives 2.1.1. Synthesis of Oxazolidinone Derivatives OxaOzxoalizdoilnidoinoesn,esa,calacslassosfofifvfiev-em-meembbeerredcycliccarrbaamaatetse,s,didsipslpaylaybiobliogliocgalicacltiavcitievsitaiensdand good antibacterial properties. Substituted oxazolidinones are not only used as substrates in organic good antibacterial properties. Substituted oxazolidinones are not only used as substrates in organic synthesis, but also as chiral auxiliaries in asymmetric synthesis [18]. In particular, some synthesis, but also as chiral auxiliaries in asymmetric synthesis [18]. In particular, some oxazolidinones oxazolidinones can be used as the core unit of antibacterial agents, such as toloxatone, linezolid and can be used as the core unit of antibacterial agents, such as toloxatone, linezolid and tedizolid [19]. Oxazolidinones can be prepared through the intramolecular nucleophilic cyclization of propynyl Novel strategiesPDF Image | Catalytic Conversion of Carbon Dioxide through C-N Bond
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