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Fu et al. In situ Catalytic Transformation SCHEME 12 | FLPs employed in CO2 capture and transformation. SCHEME 13 | Homogeneous dinuclear Zn or Mg catalysts used for the production of poly(cyclohexene carbonate). Although a plethora of CO2 absorbents has been developed and valuable products can be obtained from the resulting CO2 adducts by different strategy, however, the cost and feasibility must be considered from the viewpoint of industrial application. With this in mind, amines and ionic liquids are considered as promising absorbents for the CCU strategy. For amine absorbents, their features of high absorbing capacity and comerical availability are attractive for industrial application. Besides, the CO2 adducts derived from amines and CO2 are non-volatile liquids or solids, which can be used as starting materials instead of the volatile amines and CO2 gas to develop the gas free progress. For ionic liquid- based CO2 absorbents, the acceptable cost, tunable structure as well as their high CO2 capture capacity make them competent to the commercial CCU process. Moreover, the ionic liquids are nonvolatile and the corrosion of equipment can be avoided by subtly design the structure of ionic liquids, all of which can facilitate the industryoperability. In summary, the CO2 capture and in situ catalytic transformation is still in its infancy. We hope this review can inspire the extensive research on CO2 capture and in situ transformation, which will benefit for the design of efficient CO2 capture and utilization system (CCU) and realize the Frontiers in Chemistry | www.frontiersin.org 12 July 2019 | Volume 7 | Article 525PDF Image | CO2 Capture and in situ Catalytic Transformation
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