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In order to develop IL-based technology for CO2 separation, research work needs to be carried out from experimental measurements to modeling as well as process simulation and evaluation. In the past decades, more and more ILs with functionalized cations and anions have been synthesized in the laboratory. The thermo-physical properties (e.g. density, viscosity and surface tension) of conventional ILs as well as the effects of cation and anion of ILs on their properties and CO2 solubility have been extensively measured experimentally. While the effects of water and other components on their properties are seldom considered. Meanwhile, modeling and process simulation can predict the property of ILs, calculate the energy demand as well as estimate the capital and investment cost of the process, but the research work on the thermodynamic modeling of novel ILs and energy analysis is relatively few, and the process simulation for CO2 separation from a specific gas mixture as well as the performance evaluation of ILs on CO2 separation are still limited. Therefore, a systematic study is needed to develop IL-based technology for CO2 separation. 1.4 Objectives and outline The overall objective of this work is to perform a systematic study from experimental measurement, thermodynamic modeling to process simulation in order to develop IL-based technology. The specific objectives are: To evaluate the available experimental gas solubilities and properties of the conventional ILs; To measure thermo-physical properties of novel ILs and their gas solubility with the consideration of water effect; To perform thermodynamic modeling for representing the properties of ILs and the gas solubility in ILs; To conduct thermodynamic study for analysing energy demand for CO2 separation; To perform process simulation and evaluate the performance of ILs on CO2 separation from biogas as a case study. Figure 1.3 illustrates the flow chart of this thesis. Within the research framework, firstly, the CO2 solubility in the conventional ILs and their properties were surveyed, evaluated and 5PDF Image | CO2 Separation with Ionic Liquids
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