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Table 4.8. The NRTL binary parameters. Component i CO2 CH4 CO2 CH4 CO2 CH4 CO2 CH4 CO2 CH4 CO2 CH4 H2O H2O CO2 Component j [hmim][Tf2N] [hmim][Tf2N] [bmim][Tf2N] [bmim][Tf2N] [bmim][PF6] [bmim][PF6] ChCl/Urea ChCl/Urea [Amim][HCOO] [Amim][HCOO] H2O H2O ChCl/Urea [Amim][HCOO] CH4 mij mji 0.51 1.58 -5.5 11.21 4.5 0.82 -0.066 -1.34 -0.66 3.34 -1.54 -0.04 0.50 -4.48 39.50 0 -10.41 20.54 -5.58 13.77 10.06 10.06 0 0 1.613 -0.48 -19.48 4966.8 17.023 -7.3085 nij nji -253.82 -433.01 704.57 -1884.2 -640.52 -715.34 250.87 153.62 982.75 -1506.6 -503.33 -97.95 -1236.1 3032.6 -10000 0 2101.6 -4417.0 177.98 -1786.0 -3268.1 -3268.1 1948.87 562.113 -538.95 134.90 -16.235 3422.9 8.7759 67.012 cij= cji 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.3 0.2 0.2 0.1 4.3.2 Biogas upgrading using ILs The process simulation for biogas upgrading was conducted in Aspen Plus. The process is illustrated in Figure 3.2. For the conventional ILs, due to the low vapor ILs, the solvent was regenerated by decreasing pressure. The processes of biogas upgrading with [hmim][Tf2N], [bmim][Tf2N] and [bmim][PF6] were simulated, respectively. As shown in Table 4.9, the amount of recirculated solvent and the total energy demand for upgrading process follow: [bmim][Tf2N] < [bmim][PF6] < [hmim][Tf2N]. The power requirements of pump are different because of the differences on the amounts of recirculated solvents. The compression work contributes 60-65% to the total energy demand. conceptual pressure of 41PDF Image | CO2 Separation with Ionic Liquids
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