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[Amim][HCOO] decreased with increasing water concentration, but the influence was not notable at high water concentrations. The density and viscosity of dry [Amim][HCOO] were correlated by empirical equations and then the excess molar volumes and viscosity deviations were further calculated from the experimental density and viscosity of aqueous [Amim][HCOO]. It was found that the ideal mixing rule cannot be used to predict the properties of the aqueous [Amim][HCOO], and the quadratic mixing rule was used to correlate the experimental density and viscosity. The CO2 and CH4 solubilities in dry [Amim][HCOO] and the CO2 solubility in aqueous [Amim][HCOO] were modeled by the NRTL- RK model. The Henry’s constant was found as a very important parameter in terms of accurate modeling and had to be adjusted in the data fitting. The model parameters can be implemented into the commercial software to perform the process simulation for CO2 separation. Acknowledgement The authors thank the financial support from Swedish Research Council and Swedish Energy Agency. Moreover, the Kempe Foundations and the Bio4Energy programme are acknowledged. References [1] Meehl GA, Washington WM, Collins WD, Arblaster JM, Hu A, Buja LE, et al. How much more global warming and sea level rise? Science. 2005;307:1769-72. [2] Kenarsari SD, Yang D, Jiang G, Zhang S, Wang J, Russell AG, et al. Review of recent advances in carbon dioxide separation and capture. Rsc Advances. 2013;3:22739-73. [3] Koornneef J, van Breevoort P, Hamelinck C, Hendriks C, Hoogwijk M, Koop K, et al. Global potential for biomass and carbon dioxide capture, transport and storage up to 2050. International Journal of Greenhouse Gas Control. 2012;11:117-32. [4] Pennline HW, Luebke DR, Jones KL, Myers CR, Morsi BI, Heintz YJ, et al. Progress in carbon dioxide capture and separation research for gasification-based power generation point sources. Fuel Processing Technology. 2008;89:897-907. [5] http://www.gizmag.com/ionic-liquid-co2-emissions-control/11105/. [6] Blanchard LA, Hancu D, Beckman EJ, Brennecke JF. Green processing using ionic liquids and CO2. Nature. 1999;399:28-9. [7] Seddon KR, Stark A, Torres M-J. Influence of chloride, water, and organic solvents on the physical properties of ionic liquids. Pure and Applied Chemistry. 2000;72:2275-87.PDF Image | CO2 Separation with Ionic Liquids
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