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Figure 4. CH4 partial pressure of ChCl/Urea (1:2)-CH4 system. Symbols, experimental data (Xie et al.46); Curves, model correlation. 2.2.5. Properties and Vapor-Liquid equilibrium (VLE) of ChCl/Urea (1:2)-H2O binary system. According to the work of Zhang et al.,43 VLE data, excess enthalpy and heat capacity can be used to determine the NRTL binary parameters including their temperature dependencies. No excess enthalpy of the ChCl/Urea (1:2)-H2O binary system is available, thus, their VLE data47 and heat capacity38 were used to obtain the NRTL binary parameters. The regressed NRTL parameters are summarized in Table S4. The ARDs for the vapor pressure and heat capacity were 5.1 % and 3.7 %, respectively. The comparisons of the vapor pressure and the heat capacity are illustrated in Figures 5 and 6. The calculated vapor pressure agreed with the experimental data very well, and the deviation increased slightly with increasing temperature and increasing mole fraction of ChCl/Urea (1:2). The model also provided satisfactory representation of the heat capacity, and the deviation became larger with increasing mole fraction of water. It showed that the model with the fitted parameters and the mixing rules in Aspen Plus can be used to correlate these properties reliably. Figure 5. Vapor pressure of ChCl/Urea (1:2)-H2O system. xChCl/Urea (1:2) is the mole fraction of ChCl/Urea (1:2). Symbols, experimental data (Wu et al. 47); Curves, model correlation. 11PDF Image | CO2 Separation with Ionic Liquids
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