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• Designing catalytic sites in synthetic and biological responsive matrices with enhanced cat- alytic performance (compared to the current state-of-the art synthetic and biological cata- lysts) in a laboratory environment (TRL 3) by optimization of process variables (e.g. the rates for proton and electron transfer at the interfaces with the molecular catalytic site and the catalytic conversion rates of the small molecules) >10-year goals: • Validation of molecular compartments covering DPs and exploration of their self-assembly into responsive matrices, their optimization at interfaces between compartments, self-repair, and regulation of arrays of responsive matrices to gain a better understanding of how to maximize productive energy gradients while minimizing recombination losses • Boosting (photo)catalysis with tandem devices that operate on a laboratory scale with a photochemical current of 16 mA/cm2 under AM 1.5 irradiation, corresponding to using 70% of incoming photons (TRL 4) • Validating selected molecular compartments and responsive matrix self-assemblies under rel- evant field conditions (TRL 5) • Major cross cutting initiative: translation of key biological catalysis concepts to optimized devices to merge the best of homogeneous, heterogeneous and biological processes. 7.4.2 Developing microbial cell factories for solar energy conversion to fuels and chemicals and valorization of upstream products for feeding into the bio-based production stream 1-year goals: • Genome mining for novel enzymes with either improved catalytic function or novel reactivities. • Quantum modelling of electron- and proton-transfer processes to establish a selection criterion for the design of metabolic sinks • Integration of new control systems based on predictable models (e.g. machine learning) for phototrophic cultivation using natural sunlight • Construction of an outdoor plant at TRL 8 for the production of organic acids (e.g. Photanol) 5-year goals: • Exploration, selection, and characterization of robust strains and enzymes to be used as starting points in bioengineered systems 76PDF Image | sustainable production of fuels and chemicals
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