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Acknowledgements I would like to express my sincere gratitude to my advisors and colleagues who made this work possible. This research was conducted partly in New York at the Earth & Environmental Engineering Department and the Lenfest Center for Sustainable Energy at Columbia University and partly in Denmark at the Fuel Cells and Solid State Chemistry Division at Risø National Laboratory for Sustainable Energy. I was lucky to find two equally enjoyable research groups and learn from and contribute to both. The acknowledgements for the two sides of the collaboration are given in two columns. I thank the following people for giving me knowledge and insight, and lending their expertise and time, at various stages of the research: At Columbia Klaus Lackner — for making it all happen; for teaching me about all aspects of energy conversion and sustainability; for teaching me how to think, in your perhaps indescrib- able way of looking at complex things and honing in on unique important aspects, how to use basic physical principles, and the value of order-of-magnitude comparisons and logical arguments over precise accounting; for the many insightful discussions about carbon management and energy systems; and for giving me the opportunity and freedom to pursue this research path. Alan West — for teaching me about electrochemistry and electrode kinetics modeling; for helping me to focus the experimental studies; and for generously giving me space in your lab to set up and conduct preliminary high temperature experi- ments. Paul Duby — for introducing me to electro- chemistry; for teaching me how to work in a lab and supporting my initial interest in aqueous CO2 electrolysis experiments; for giving me a foundation in thermodynamics and chemistry; and for guidance and support throughout. At Risø Mogens Mogensen — for teaching me about high temperature electrochemistry; for invit- ing me to your excellent lab and research group to conduct my experimental work in the presence of some of the greatest expertise in the field; for the many valuable discussions lending me your deep understanding of elec- trochemistry and materials; for encouraging, supporting and guiding my experiments while also giving me plenty of room to explore. Sune Ebbesen — for the initial daily help and teaching me electrochemical cell character- ization techniques; for the many insightful discussions about experiments and electro- chemistry; for being receptive to work with an unknown guest PhD studentand having a productive time working together. Bhaskar Reddy Sudireddy — for teaching me theory and lab procedures for preparing ceramic materials and characterization their properties, and for the nice cooperation in the materials study. Konrad Tarka — for help with materials synthesis and a productive ―Summer of Molybdates and Titanates.‖ Best of luck on your master’s project! xivPDF Image | Electrolysis of CO2 and H2O
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