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surface area promoted the reaction of large molecules. Srivastava et al. [47] prepared the nanosheet MFI zeolite by combining two structure directing agents of tetrapropylammonium bromide (TPABr) and C18-6-6 (Figure 5). TPABr induced the formation of microporous structure of MFI zeolite. The long hydrophobic chains of C18-6-6 facilitated the ordered stacking of microporous zeolite layers to Cpartoaldysutsc2e01n7a, 7n,o3s67heet-like morphology. Besides, it restrained the excessive growth of zeolites7 oafn3d1 induced the formation of inter-crystalline mesopores. Figure 4. SEM images of as-made samples: BCPh-4-6-6 (a); BCPh-6-6-6 (b,c); BCPh-8-6-6 (d); BCPh-10-6-6 (e); and Figure 4. SEM images of as-made samples: BCPh-4-6-6 (a); BCPh-6-6-6 (b,c); BCPh-8-6-6 (d); BCPh-10-6-6 (e); BCPh-12-6-6 (f), all showing the formation of single-crystalline zeolite nanosheets with 90 °C rotational and BCPh-12-6-6 (f), all showing the formation of single-crystalline zeolite nanosheets with 90 ◦C boundary. The scale bars in (a–f) represent 1 mm, 500 nm, 100 nm, 500 nm, 1 mm and 1 mm, rotational boundary. The scale bars in (a–f) represent 1 mm, 500 nm, 100 nm, 500 nm, 1 mm and 1 mm, respectively [42]. Copyright Nature Publishing Group, 2014. The nanosheet MFI zeolite with high BET surface area and mesopore volume was synthesized with C22-6-6 and ethanol as structure-directing agents. The conversion increased by 26% with less carbon deposition in supercritical catalytic cracking of n-dodecane, due to high diffusion efficiency and better accessibility of acid sites resulting from the superior morphology property [44]. TPAOH was also selected as a second SDA to prepare the nanosheet MFI with different morphology and texture properties by changing its concentration [45]. The morphology of the synthesized nanosheet MFI zeolite changed from intertwined, to house-of-cards-like, and to dense packing plates with the increase of TPAOH concentration. The textural property increased firstly and then respectively [42]. Copyright Nature Publishing Group, 2014.PDF Image | Strategies to Enhance the Catalytic Performance of ZSM-5
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