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Catalysts 2015, 5 2233 case also, as with H-beta zeolites, the greatest activity was obtained with the intermediate SAR ratio. Overall, however, the activity was not much affected by the Si/Al ratio. (A) (B) (C) (D) (E) FigFuirgeur5e. 5P.hePnhoelnboelnzboeynlzaotiyolnatwiointhwBitAh:BpAhe:npohlecnonlvceorsnivoenrsbiaosnedbaosnedreoanctiroenacttiimone (A) time (A) and selectivity to phenylbenzoate (B), to p-hydroxybenzophenone (C), and selectivity to phenylbenzoate (B), to p-hydroxybenzophenone (C), and ◦ selectivity ratio between p- and o-hydroxybenzophenone. Catalysts: H-Y zeolites. between p- and o-hydroxybenzophenone. Catalysts: H-Y zeolites. and o-hydroxybenzophenone (D) based on phenol conversion at T = 190 C. (E): o-hydroxybenzophenone (D) based on phenol conversion at T = 190 °C. (E): selectivity ratio With these catalysts, also, PB was the only primary product, and the formation of HBPs occurred by Even when we changed the BA/phenol molar ratio (Figure 6), the highest the consecutive transformation of the ester. However, the selectivity to HBPs was lower than that shown overall selectivity to HBPs achieved was not higher than 32%. An excess of phenol, with H-beta zeolites, even with the more active H-Y sample. Therefore, H-Y zeolites were also poorly in experiments carried out at a BA/phenol molar ratio equal to 0.5 and 0.16, should efficient in the consecutive transformation of PB into HBPs; this is particularly apparent with the sample be kinetically unconducive to an intermolecular transformation of PB to HBPs 128PDF Image | Zeolite Catalysis
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