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HIGHBIO2 PROJECT PUBLICATION mainly for CO2 solubility in ILs. However, the application of IL-based technology for CO2 recovery requires knowledge of CO2 solubility, the effect of other components on CO2 solubility, the properties, the heat and mass transport rate as well as process evaluation. Therefore, a tremendous gap exists between new technology development and implementation. The work in our research group aims to perform a systematic research from experimental data measurement, model development to process simulation and integration in order to promote IL-based technology development and application. In this study, our group’s research work on the following areas is summarized: the survey of available experimental data, the model development, and new experimental data measurements. In addition, we provide the corresponding prospects of developing and utilization IL-based technology for CO2 separation. Available experimental data Experimental data plays an important role in model development and verification. Pure-component or binary model parameters need to be obtained from the fitting to available experimental data, and model performance needs to be verified by the experimental data. Having reliable experimental data is a prerequisite for model parameterization and verification, and model development provides more information over a wide range of conditions and gives insights into understanding interactions on a molecular level. The combination of reliable experimental data and model development is a good way in research. In this section, the gas solubility in imidazolium-based ILs is summarized. The CO2 solubility in ionic liquids such as [Cnmim][BF4] (1-alkyl- 3-methylimidazolium tetrafluoroborate) and [Cnmim][PF6] (1-alkyl-3- methylimidazolium hexafluorophosphate), and [Cnmim][Tf2N] (1-alkyl- 3-methylimidazolium bis(trifluoromethylsulfonyl)imide), n = 2, 4, 6, 8 has been measured extensively and collected in the database IL Thermo (NIST, 2006; Ji et al., 2012). However, most of the experimental data is for C4mim- based ILs. For some ILs, the CO2 solubility data is still limited. For example, there are only two sources for [C6mim][PF6] and [C8mim][Tf2N], and only one source for [C2mim][PF6] and [C8mim][PF6]. New experimental data is still needed, and a predictive model is highly desirable. 68PDF Image | BIOMASS TO ENERGY AND CHEMICALS HighBio2 Project Publication
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