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12 1 Supercritical Carbon Dioxide for Sustainable Polymer Processes Fig. 1.10 Development trajectory of an emerging technology [63]. and pharmaceuticals industry because of additional marketing advantages, such as the GRAS (generally regarded as safe) status. However, the fact that DuPont is commercializing the production of fluoropolymers in scCO2 [66] illustrates the application possibility of supercritical fluid technology in polymer processes also. In addition, the long-existing ldPE tubular process (ca. 250 MPa, 600 K) proves that a high-pressure polymerization process performed on a large scale can survive in a highly competitive field. Nevertheless, the progress made in research today will enable the develop- ment of sustainable industrial polymer processes for the future. For this reason, the various subjects in this book have been addressed from an engineering point of view. The book is divided into three parts: an overview of polymer fun- damentals, polymerization reactions, and polymer processing in supercritical carbon dioxide. It covers topics in a multidisciplinary approach starting in Part I with thermodynamics (Chapter 2), mass and heat transfer (Chapter 3), polymer- ization kinetics (Chapter 4), and monitoring (Chapter 5). In Part II, different types of polymerization processes (Chapters 6 to 9) will be discussed, and Part III describes the possibilities for polymer post-processing (Chapters 10 and 11), including reactive extrusion (Chapter 12), end group modification (Chapter 13), and residual monomer removal (Chapter 14). Notation Pc critical pressure Q quadrupole moment Tc critical temperature Tg glass transition temperature a polarizability Cij potential energy [MPa] [erg1/2 cm5/2] [K] [K] [cm3] [J]PDF Image | Supercritical Carbon Dioxide for Sustainable Polymer Processes
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