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Figure Page FIGURES 1. Releasing the pressure on a bottle of soda pop causes dissolved CO2 to leave the liquid—slowly under normal conditions, or spectacularly if the transfer is promoted with an appropriate accelerating additive.1 ..........................................9 2. Absorption gas separation using temperature-swing gas separation takes advantage of the high solubility of target gas at low temperature and lower solubility at high temperature. .................................................................................9 3. The adsorbent material can be designed to be highly size- and shape- selective..................................................................................................................19 4. Model nanoporous oxygen carriers........................................................................21 5. Schematic of a membrane separating a mixture of molecules...............................25 6. Comparison of a membrane unit with a conventional separation process (i.e., amine absorption system) for removing CO2 from natural gas. ............................26 7. Gas sizes (D), critical temperature (Tc), and common order of permeability coefficients of gas molecules in polymers. ............................................................29 8. Photomicrograph of a hollow fiber gas separation membrane showing the graded porosity in the wall of the fiber and the ultrathin (~100 nm) separating layer at the outer wall of the fiber. .......................................................30 9. Permeability/selectivity tradeoff as illustrated for the separation of mixtures of hydrogen and nitrogen.......................................................................................31 10. Effect of membrane thickness and time on gas permeability properties of Matrimid®, a glassy polymer. ................................................................................32 11. Forming asymmetric hollow fiber membranes involves solution processing of polymers to a highly nonequilibrium state. .......................................................33 12. Snapshots (top and side views) of the solution–air interface of 1.2 M aqueous sodium halides from molecular dynamics simulations and number density profiles of water oxygen atoms and ions plotted vs distance from the center of the slabs in the direction normal to the interface, normalized by the bulk water density. .................................................................................................40 13. Schematic of CO2 selectively isolated by dissolving in a liquid and its subsequent chemical reaction with absorbent, A...................................................43 14. Systematic methodology for developing optimal liquid-solvent separation processes. ...............................................................................................................52 15. Currently used and researched sorbents and their capacity as a function of temperature. ...........................................................................................................58 16. Atomic simulation of 3D ordered architectures (a) and disordered architectures (b) and (c). ........................................................................................60 17. Multivariate MOF-5 structure with eight different functionalities. .......................60 18. Top: Quaternary structures of deoxyhemoglobin (T state) and oxyhemoglobin (R state), which demonstrate considerable structural change upon uptake of an O2 molecule. .............................................................................65 vPDF Image | 2020 Carbon Capture
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