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and modulating the heat of adsorption. For example, one might consider coating a material that incorporates iron or nickel oxide onto carbon to enable magnetic manipulation/triggering of the sorbent. The discussion in this PRD is meant to inspire the development of wholly new concepts for solid sorbent materials. Such materials with improved structure and functionality will require the development of alternative synthesis routes guided by a fundamental understanding of chemical and physical processes involved in gas sorption/release. Scientific Questions and Opportunities • A key fundamental question revolves around the roles of pore structure and pore size for efficient sorbents. Answering it requires a rethinking of traditionally held views on effective sorbents. Can systems with a controlled pore size and structure be used as models to elucidate gas–solid interactions? • Tailoring the surfaces of solid sorbents has enormous potential for improving gas uptake and release. Can the curvature of a particle be tuned to obtain reversible, high-specificity gas sorption? Can surface functionalities be incorporated on surfaces and in pores to enhance sorption and improve selectivity while maintaining long-term cyclability? Can heterostructures based on highly porous carbon, MOFs, polymers, and other porous networks provide another route to improved gas separation schemes? • Advances in nanoscience and technology have provided new tools for synthesizing materials. Can nanoscience provide novel modalities of control over structure and properties to enhance gas uptake/release strategies? Can new classes of materials be synthesized by self-assembly or top-down approaches? Potential Impact Maximizing the density of gas sorption within the adsorbent volume, controlling the mechanisms and rates of adsorption and release, and developing new materials with higher selectivity will lead to drastically improved capacity and energy efficiency for targeted gas adsorption and desorption throughout the carbon cycle. Success in the discovery of new material architectures will require interdisciplinary teams to develop new sorbent architectures,which will involve close coupling of theory, synthesis, and characterization. Development of new solid sorbents with improved selectivities will have a broad impact in many areas beyond carbon capture, including gas purification and emission control processes used across industry. The new generation of complex nanostructured material architectures developed for targeted gas sorption may impact other energy-related applications, including catalysis, energy storage, and water desalination References 1. S. Choi, J. H. Drese, and C. W. Jones, “Solid adsorbent materials for carbon dioxide capture from large anthropogenic point sources, ChemSusChem 2(9), 796–854(2009). 2. H. K. Chae, D. Y. Siberio-Perez, J. Kim, Y-B. Go, M. Eddaoudi, A. J., Matzger, M. O’Keeffe, and O. M. Yaghi, “A route to high surface area, porosity and inclusion of large molecules in crystals,” Nature 427, 523–27 (2004). 61PDF Image | 2020 Carbon Capture
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