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Figure 26. Light-driven molecular impellers: molecular rotors inside mesoporous silicon are used to generate fluid forces that can transport dye molecules through these narrow channels. Source: J. Lu, E. Choi, F. Tamanoi, and J. I. Zink, “Light-activated nanoimpeller-controlled drug release in cancer cells,” Small 4(4) 421–426 (2008). Copyright Wiley- VCH Verlag GmbH and Company KGaA. Reproduced with permission. These examples provide a strong motivation for exploring the potential of designing a new generation of materials for membranes, solid adsorbents, and liquid absorbents that could greatly reduce the cost associated with carbon capture processes. These next-generation materials will be realized only with the capability to develop new materials with tailored structures and functionalities that respond to specific stimuli. Developing this capability will require a fundamental understanding of the interactions of applied stimuli with materials, and of the associated physical and chemical interactions of a targeted gas molecule/ion with the new materials, both with and without the effect of the applied stimulus. Advanced characterization and modeling tools are required to guide the synthesis and discovery of new materials and mechanisms that can be incorporated into revolutionary processes for efficient gas separation. Research Directions New classes of gas separation materials are needed that can harness driving forces (stimuli) to cause efficient separation of a targeted gas molecule or ion from a complex mixture. Smart materials that can be switched between capture and release conditions encompass a wide range of systems in which the stimulus causes a strong alteration of the chemical or physical interactions of the material with the target species (see the PRD “Cooperative Phenomena for Low Net Enthalpy of Cycling”). Such switching needs to result in a sufficient change in the binding affinity or capacity for targeted species without requiring a large energy input. Outlined in the following paragraphs are examples intended to inspire new approaches to designing materials or processes that would dramatically reduce the energy requirement for targeted gas capture and release. 80PDF Image | 2020 Carbon Capture
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