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new separation approaches could also make these processes more selective and more energy- efficient. Further, the new materials and processes developed as part of this research could impact a broad range of other applications in which smart, switchable materials are needed, including novel sensors, drug delivery systems, and others. References 1. D. Tanaka, K. Nakagawa, M. Higuchi, S. Horike, Y. Kubota, T. C. Kobayashi, M. Takata, and S. Kitagawa, “Kinetic gate-opening process in a flexible porous coordination polymer,” Angew. Chem. Int. Ed. 47, 3914–3918 (2008). 2. J. Lu, E. Choi, F. Tamanoi, and J. I. Zink, “Light-activated nanoimpeller-controlled drug release in cancer cells,” Small 4(4) 421–426 (2008); W. R. Dichtel, O. Š. Miljanić, W. Zhang, J. M. Spruell, K. Patel, I. Aprahamian, J. R. Heath, and J. F. Stoddart, “Kinetic and thermodynamic approaches for the efficient formation of mechanical bonds,” Acc. Chem. Res. 41, 1750–1761 (2008). 3. G. Férey and C. Serre, “Large breathing effects in three-dimensional hybrid matter: Facts, analyses, rules, and consequences,” Chem. Soc. Rev. 38, 1380–1399 (2009). 4. J. Seo, R. Matsuda, H. Sakamoto, C. Bonneau, and S. Kitagawa, “A pillared-layer coordination polymer with a rotatable pillar acting as a molecular gate for guest molecules,” J. Am. Chem. Soc. 131, 12792–12800 (2009). 5. R. F. Khairutdinov and J. K. Hurst, “Light-driven transmembrane ion transport by spiropyran−crown ether supramolecular assemblies,” Langmuir 20(5), 1781–1785 (2004). 6. N. K. Mal, M. Fujiwara, and Y. Tanaka, “Photocontrolled reversible release of guest molecules from coumarin-modified mesoporous silica,” Nature 421, 350–353 (2003). 7. K. L. Mulfort, T. M. Wilson, M. R. Wasielewski, and J. T. Hupp, “Framework reduction and al kali-metal d oping of a t riply catenating m etal-organic f ramework enhances an d then diminishes H2 uptake,” Langmuir 25, 503–508 (2009). 8. D. Li, M. H. Zhao, J. Garra, A. M. Kolpak, A. M. Rappe, D. A. Bonnell, and J. M. Vohs, “Direct in situ determination of the polarization dependence of physiosorption of ferroelectric surfaces,” Nature Mater. 7, 473–477 (2008). 9. B. D. Chandler, G. D. Enright, K. A. Udachin, S. Pawsey, J. A. Ripmeester, D. T. Cramb, and G. K. H. Shimizu, “Mechanical gas capture and release in a network solid via multiple single-crystalline transformations,” Nature Mater. 7, 229–235 (2008). 10. M. A. C. Stuart, W. T. S. Huck, J. Genzer, M. Müller, C. Ober, M. Stamm, G. B. Sukhorukov, I. Szleifer, V. V. Tsukruk, M. Urban, F. Winnik, S. Zauscher, I. Luzinov, and S. Minko, “Emerging applications of stimuli-responsive polymer materials,” Nature Mater. 9 101–113 (2010). 84PDF Image | 2020 Carbon Capture
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