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Annex I: Properties of CO2 and carbon-based fuels 387 Figure AI.2 Variation of CO2 density as a function of temperature and pressure (Bachu, 2003). Figure AI.3 Vapour pressure of CO2 as a function of temperature (Span and Wagner, 1996). water also decreases with increasing water salinity by as much as one order of magnitude (Figure AI.7). The following empirical relation (Enick and Klara, 1990) can be used to estimate CO2 solubility in brackish water and brine: wCO2, b = wCO2, w · (1.0 – 4.893414 · 10−2 · S + 0.1302838 · 10−2 · S2 – 0.1871199 · 10−4 · S3) (1) where wCO2 is CO2 solubility, S is water salinity (expressed as total dissolved solids in % by weight) and the subscripts w and b stand for pure water and brine, respectively. A solid hydrate separates from aqueous solutions of CO2 that are chilled (below about 11oC) at elevated pressures. A hydrate is a crystalline compound consisting of the host (water) plus guest molecules. The host is formed from a tetrahedral hydrogen- bonding network of water molecules; this network is sufficiently open to create pores (or cavities) that are large enough to contain a variety of other small molecules (the guests). Guest molecules can include CH4 and CO2. CO2 hydrates have similar (but not identical) properties to methane hydrates, which have been extensively studied due to their effects on natural gas production and their potential as future sources of hydrocarbons.PDF Image | CARBON DIOXIDE CAPTURE AND STORAGE
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