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5-1 Left: Experimental Configuration. Upper Right: Deposition of poly L-lysine (PLL) layers. Lower Right: Data showing charge inversion of positive PLL layers on a negative silica surface with increasing concen- trationofKClinwater.[83]....................... 117 5-2 Diagram of the geometry used for the model. Domain I contains a positively charged polymer (PLL) that has been deposited on the silica surface. .................................. 118 5-3 Difference in potential between surfaces with and without PLL as a function of KCl concentration with PLL of molecular weights of 150000- 300000 g/mol using the traditional Debye-Huckel model, taking in ac- count dielectric constant differences between domains I and II. . . . . 125 5-4 Difference in potential between surfaces with and without PLL as a function of KCl concentration with PLL of varying molecular weights. Heavy refers to a molecular weight of 150000-300000 g/mol, medium refers to a molecular weight of 30000-70000 g/mol, and light refers to a molecular weight of 4000-15000 g/mol. Overall, we observe that the absolute value of the difference in potential becomes smaller as the molecularweightdecreases. ....................... 126 5-5 Difference in potential as a function of KNO3 concentration for PLL ofamolecularweightof150000-300000g/mol. . . . . . . . . . . . . . 128 5-6 Difference in potential as a function of MgCl2 concentration for PLL ofamolecularweightof150000-300000g/mol. . . . . . . . . . . . . . 129 5-7 Difference in potential between surfaces with and without PLL as a function of KCl concentration with PLL of varying molecular weights using the Pincus relation for layer thickness. Heavy refers to a molec- ular weight of 150000-300000 g/mol, medium refers to a molecular weight of 30000-70000 g/mol, and light refers to a molecular weight of 4000-15000g/mol. ............................ 131 18PDF Image | Shock Electrodialysis for Water Purification and Electrostatic Correlations
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