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Figure 5-10: Difference in potential between surfaces with and without PLL as a function of KCl concentration with PLL of varying molecular weights using the Pin- cus relation for layer thickness and incorporating the Born solvation energy at the interface. Heavy refers to a molecular weight of 150000-300000 g/mol, medium refers to a molecular weight of 30000-70000 g/mol, and light refers to a molecular weight of 4000-15000 g/mol. (relative to the same concentration of KNO3) also causes the bulk dielectric constant to be lower (i.e. increases the difference in dielectric constants between domain I and II). Overall, the biggest change in parameters that we observe is that the dielectric constant for domain I for MgCl2 decreased by 11% and that we see the trends between the various electrolytes change a little to where MgCl2 is now the electrolyte that forms the thickest and least dense polymer layer, which is significantly driven by the additional effective charge density created by the solvation energy. 5.3.6 Potential Profiles In addition to comparing the new model’s performance to experimental data, some interesting observations can also be made by simply looking at the potential pro- files predicted by the new model, especially, since traditional models simply predict an exponentially decaying potential. Figures 5-13 – 5-16 show the potential profile obtained under various conditions. First, it is interesting to not that at low con- 134PDF Image | Shock Electrodialysis for Water Purification and Electrostatic Correlations
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