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Nanomaterials 2020, 10, x FOR PEER REVIEW 7 of 10 can be identified and would originate due to the dissociation of water. The second positive system 33 Naenmomiastserioianls o20f2N0,21(0C, 87Π4μ to B Πg) can be seen in low intensity at 337, 357 and 380 nm. The nitrogen lin7eosf 10 may occur due to the dissolved nitrogen in the aqueous precursor solution. Moreover, oxygen emission lines can be found in 777 nm and 844 nm. Identified spectral lines for argon are included in in 777 nm and 844 nm. Identified spectral lines for argon are included in Table 2 including transitions, Table 2 including transitions, relative intensities, and energy levels. relative intensities, and energy levels. Table 2. Observed optical emission spectroscopy (OES) data of the argon emission spectral lines. Table 2. Observed optical emission spectroscopy (OES) data of the argon emission spectral lines. Transition, initial energy levels (Ei) and final energy levels (Ef) taken from Ref [10]. Transition, initial energy levels (Ei) and final energy levels (Ef) taken from Ref [10]. Wavelength (nm) Transition Relative Intensity (a.u) Relative In61te3n7s1ity (a.u) Ei (eV) Ef (eV) 1E3.3(3eV) 11.55 E (eV) if Wavelength (n6m9)6 Tran2sipt2ion 1s5 2p3 1s5 2p2 → 1s5 2p →2p51s1s5 35 2p→1s 5 2p25 1s4 2p→1s 2 2p34 1s4 707 707 715 15587 13.30 11.55 11.55 11.62 11.62 11.83 11.62 11.55 11.55 11.72 11.55 11.62 11.55 11.83 11.83 11.62 11.83 696 61,371 13.33 153,52874 131.238.30 11.55 11.55 11.55 11.62 11.62 11.83 11.62 11.55 11.55 11.72 11.55 11.62 11.55 11.83 11.83 11.62 11.83 715 727 738 750 751 763 772 795 795 801 810 811 826 841 842 852 3284 13.28 727 738 750 751 763 772 26821 13.33 801 810 811 826 841 842 852 48,875 13.09 2p→1s 34 30896 13.30 2p1 1s2 2p1 → 1s2 30,896 13.30 2p5 1s4 2p5 → 1s4 55,719 13.48 2p6 1s5 2p6 → 1s5 36,434 13.27 2p2 1s3 2p2 → 1s3 2p →2p41s1s3 43 2p→1s 6 2p64 1s4 65,549 13.17 2p→1s 74 50,477 13.15 2p7 1s4 50477 13.15 2p→1s 95 62,028 13.08 2p9 1s5 2p2 → 1s2 62028 13.08 2p2 1s2 2p3 → 1s2 61,613 13.33 2p3 1s2 2p8 → 1s4 27,474 13.30 2p8 1s4 2p4 → 1s2 61,277 13.09 2p4 1s2 The transfer of these species occurs in the plasma–liquid interface and a fraction of these species 18474 13.28 The transfer of these species occurs in the plasma–liquid interface and a fraction of these species 26,821 13.33 55719 13.48 36434 13.27 65549 13.17 65450 13.15 65,450 13.15 575,775566 131.238.28 48875 13.09 61613 13.33 27474 13.30 61277 13.09 18,474 13.28 is transported into the liquid interface. Within the gas–liquid interface, the possible reactions to is transported into the liquid interface. Within the gas–liquid interface, the possible reactions to take take part are the recombination, absorption or desorption of reactive species and the solvation of the part are the recombination, absorption or desorption of reactive species and the solvation of the electrons [34]. Due to the complex mechanisms of these chemical reactions, a number of unexplained electrons [34]. Due to the complex mechanisms of these chemical reactions, a number of unexplained questions remain regarding the plasma-induced liquid chemistry. questions remain regarding the plasma‐induced liquid chemistry. FigFuigruere5.5. OESSspsepcetcrutrmumof tohfetAhregoAnrDgoBnDDplBasDmapluassemdatoutrseadt thtoe ptreacut rtshoer sporluectiuornso(lrefts)o;lsuchtieomna(tliceft); schrepmreasteicntraetpiorensoefnthaetioDnBoDfpthlaesmDBaDasspilsatesmd sailavsesrisntaendospilavretirclneafnoormparttioicnle(rfiogrhmt)a.tion(right). ThTehseolsvoalvteadteedleecltercotnrosnasbsaobrsboerdbeidntointhoetlhiqeulidqupidenpeternaetteratfeewa fneawnonmaneotemrsetaenrds raenadctrweaictht wsoiltvhent mosolelvcuenletsmtoleicnudluescetoainduumcebearnoufmcbheermoficcahlermeaicatliorneasc[t1io2n]sin[1c2l]uisnivcleusoifvethoef rtheedurecdtiuocntionf soiflvsielrveirons ++ EqiuonastioEnqu(a1t)i.onTh(1e).rTedheoxrepdotxepnotitaelnotifalAogfA/Agg/Aigsi(s+(0+.07.9799V)),,whichmakeessththeeinisntsatnatnctacpatpurtueroefothfethe solvated electrons and synthesis of the reduced silver atoms. The atmospheric pressure plasma may have electrons with an energy level up to 20.2 eV and it is possible for the positive ions to also havePDF Image | Bactericidal Silver Nanoparticles by Plasma Processing
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