TEMPERATURE SWING ADSORPTION COMPRESSION AND MEMBRANE SEPARATIONS

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TEMPERATURE SWING ADSORPTION COMPRESSION AND MEMBRANE SEPARATIONS ( temperature-swing-adsorption-compression-and-membrane-separa )

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LIST OF FIGURES 1.1 Conceptual design of the 2 stage TSA compression subsystem . . . . . . 3 1.2 Conceptualized schematic of the membrane-integrated CO2 removal and compressionsystem ............................. 4 2.1 TypicalworkcycleofaTSAcompressionsystem . . . . . . . . . . . . . 8 2.2 Pure-component isotherm of CO2 on 5A at 25◦C. Symbols are experimen- tal data. The solid line is the equation Toth prediction. . . . . . . . . . . 13 2.3 Pure-component isotherm of CO2 on 5A at 25◦C. Symbols are experimen- tal data. The solid line is the equation Toth prediction. . . . . . . . . . . 14 2.4 Comparison of stage volume vs equilibrium pressure using 5A in both stagesandataregenerationtemperatureof473K. . . . . . . . . . . . . 17 2.5 Comparison of stage volume vs equilibrium pressure using 5A in stage 1, NaY in stage 2, and at a regeneration temperature of 473 K. . . . . . . . 18 2.6 Modeled breakthrough curve for CO2 adsorbed on 5A zeolite for various lengthsofsorbent. .............................. 20 2.7 Stage1workcapacitydiagram........................ 21 2.8 Stage2workcapacitydiagram........................ 22 3.1 Geometry of the adsorption bed used in finite element modeling. . . . . 32 3.2 Loading profile for the uniform heating model considered 30 minutes into thedesorptionhalf-cycle. .......................... 34 3.3 Loading profile for the uniform heating model considered at the end of thedesorptionhalf-cycle. .......................... 35 3.4 Loading profile for the nonuniform single heater model 30 minutes into thedesorptionhalf-cycle. .......................... 36 viii

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