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TEMPERATURE SWING ADSORPTION PROCESSES FOR GAS SEPARATION

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TEMPERATURE SWING ADSORPTION PROCESSES FOR GAS SEPARATION ( temperature-swing-adsorption-processes-for-gas-separation )

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kg) into the second monolith; hence, the second stage adsorption time is fixed to 0.11 s. Using this approach, adsorption times for the two monoliths in the second stage are fixed, thereby reducing the total number of degrees of freedom. The intermediate HTF tank contains the gaseous fraction of the component mixture separated from the HTF. Although, this staged purification scenario requires three times the mass of adsorbent and energy than the single stage case; it is possible to achieve product purities as high as 99.8% at a recovery factor of 31.6% at the end of the second stage. By reducing the amount of CO2 entering the system in the first stage, which is possible by selecting a shorter first stage adsorption time of 0.16 s, the second stage product purity can be increased to 99.9%. Figure 3.12. Implementation of the microchannel TSA-based purification process for multistage operation. Numerical values show calculated purity and product collected normalized with mass of adsorbent. 95

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TEMPERATURE SWING ADSORPTION PROCESSES FOR GAS SEPARATION

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