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using the electronic excitation mechanism is only about 25% in an experimental non- thermal electric discharge due to the high CO cost of 11.5 eV/mol. Figure 3.9 shows various simulated theoretical results including some experimental results for energy efficiency of CO2 dissociation stimulated by electronic excitation. Curves 1 and 2 represent the inclusion of singlet and triplet states, while curve 3 is of total energy efficiency with the dots showing experimental results. Figure 3.9: Electronic excitation energy efficiency [37]. 3.2.3 Thermal Discharges In thermal discharges, dissociation is achieved by a shift in thermodynamic equi- librium in the direction of CO formation. The thermal plasma simply provides the high temperatures needed for the shift to occur. Figure 3.10 shows simulated results of CO2 dissociation as a function of gas temperature at a pressure of about 120 torr (0.16 atm). For significant conversion of CO2 to CO, the gas temperature must reach at least 3000 K. These high temperature requirements actually limit the efficiency of the process. The products must be quickly quenched (at a rate on the order of 107 K/s and greater) to prevent the recombination of CO and O to produce CO2, which can be otherwise prevalent under those temperature conditions. Also, thermal 54PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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