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Figure 6.8: CO production as a function of CO2 flow. Power remains constant at 1.75 kW, while CO2 flow rate is varied from 1-12 slm for two different Ar flows of 8 and 10 slm. reaching almost 50%, while the lower conversion corresponds to the highest CO2 flow rate of 16 slm resulting in only 10%. It is no surprise that the highest conversion rate occurred for the highest value of specific energy tested, about 27 eV/mol. If higher values of specific energy were tested, no doubt conversion efficiency would continue to increase, possibly approaching 100%. However, the energy efficiency of such a case would be miniscule. Energy efficiency of CO2 conversion in this system is lower than expected, given the non-equilibrium and high electron density characteristics of atmospheric pressure surface wave discharges outlined in Section 5.1. For the lower value of Ev = 1.5 eV/mol tested here, experimental and computational results in other discharge systems reported efficiencies around 50% as previously shown in Figure 5.1, which is what was expected to be achieved in this system. Therefore the CO2 plasma must behave differently than the noble gas plasmas created with Ar, Ne, and He, whose density and temperature measurements were reported in liturature [67,88]. Plasma temperature measurements gained from OES of the CO2 discharge may provide some insight into this unexpected 116PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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