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Figure 6.9: Energy efficiency of CO2 dissociation. All operating conditions of CO2 flow rate, 1-16 slm, are displayed for all three different Ar flow rates (6 slm = •, 8 slm = , 10 slm = ) and the corresponding power levels from 1-2 kW. behavior. 6.1.3 Optical Emission Spectroscopy of the CO2/Ar Plasma 6.1.3.1 SPECAIR Temperature Evaluation Plasma temperature evaluation by OES was limited to the C2 Swan system, as already discussed in Section 5.4. Using the Ocean Optics HR4000, optical emission spectra were taken for each operating condition and compared to the simulated spectra generated by SPECAIR. While the translational temperature was assumed equivalent to the rotational temperature and did not affect the computed spectrum, the rotational, vibrational, and electronic temperatures all had significant effects on the Swan system. Figure 6.11 shows the experimental emission spectrum for the operating condition 10 slm Ar, 1 slm CO2, and 1 kW of power. Species molar fractions for this operating condition are computed from MS data and inserted into SPECAIR for spectra compu- tation. Accompanying the experimental spectrum are different results for the simulated spectrum assuming a constant electronic temperature and vibrational temperature 117PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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