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Figure 6.16: Conversion efficiency of CO2 dissociation with uncoated monolith. All operating conditions of CO2 flow rate, 1-8 slm, are displayed for two different Ar flow rates (8 slm = • , 10 slm = ) and the corresponding power levels from 1-2 kW. comparison with the pure plasma system shown in Figure 6.14. Here the electronic temperature is between 11,000-12,000 K (∼ 1 eV), whereas in the pure plasma system Tel = 14, 000 − 15, 000 K. The rotational temperature is about 500 K higher (greater than the ±100 K error in matching the simulated spectra to the experimental spectra) than the pure plasma system, reaching 6500 K. From these results it appears that the plasma has moved closer to reaching equilibrium between Tel and Tr. Consequently, Tr is also closer in equilibrium to the vibrational temperature. As already discussed, systems described by Tv ≈ Tr result in lower energy efficiency, which can explain the slight drop in efficiency with the presence of the uncoated monolith. 6.2.2 Rh/TiO2 Catalyst Test A monolith coated with Rh/TiO2 was inserted into the discharge at the same location as the uncoated monolith. All operating conditions for CO2 and Ar flow rates are identical to the conditions tested with the uncoated monolith, with only a few slight variations in MW power for 6 and 8 slm CO2. Similarly, a new catalyst-coated 127PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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