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Figure 6.18: Energy efficiency of CO2 dissociation in the plasma/catalyst system. All operating conditions of CO2 flow rate, 1-8 slm, are displayed for two different Ar flow rates (8 slm = • , 10 slm = ) and the corresponding power levels from 1-2 kW. the pure plasma system. Unfortunately the Rh/TiO2 catalyst material had a negative effect on the CO2 conversion process to CO. 6.2.2.2 Plasma/Catalyst Temperatures Perhaps analysis of the optical emission spectra can provide some insight into how the plasma properties are affected by the presence of the catalyst material. Figure 6.20 gives results for the plasma temperature measurements taken from analysis of the C2 system. The electronic temperature remains almost constant for all operating conditions at 12,000 K (∼ 1 eV). Similarly, vibrational temperature remains right around 7700 K until low values of specific energy are reached where Tv increases to 8000 K. Rotational temperatures are also constant around 6500 K until increasing to almost 7000 K at low specific energy values. The temperature results are not significantly different from the plasma/monolith system shown in Figure 6.17, indicating there must be another influence causing lower efficiencies in this system. 129PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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