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conversion efficiency, in contrast to the experimental results that showed no effect of Ar flow rate on dissociation. This Ar flow rate trend is most likely an artifact of the simulation’s method for calculating initial species density. The user defines a total gas flow rate and the initial molar fractions of each gas species. The program also assumes a constant pressure throughout the simulation. Thus at constant CO2 gas flow rate, an increase in Ar flow rate decreases the CO2 molar fraction and effectively the density. At constant power, this results in the equivalent effect of decreasing CO2 flow rate into the system. As already shown in the experimental results, a decrease in CO2 flow rate increases conversion efficiency as the energy distribution increases per molecule. These computational results may suggest that total pressure does not remain constant in the discharge tube. (a) (b) Figure 6.26: Computational results for operating conditions outside the experimental test plan: a) CO2 conversion as a function of Ar flow rate with constant power of 1.75 kW and constant pressure of 760 torr, b) CO2 conversion as a function of pressure with constant power of 1 kW and constant Ar flow rate of 10 sccm. Figure 6.26b demonstrates the effects of pressure on the simulated conversion efficiency. The pressure is varied from 760 torr to 1 torr at constant MW power of 1 kW and constant Ar flow rate of 10 sccm. For both constant input flow rates 137PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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