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(a) (b) Figure 6.27: Summary of efficiency results for all three experiments: • for the pure plasma system, for the plasma/monolith system, and for the plasma/catalyst system. the shift towards further equilibrium between Tv and Tr. The uncoated monolith and the catalyst-coated monolith must be affecting the plasma, particularly at high CO2 flow rates. It is probable that the geometry of the monolith caused a physical change in the plasma by impeding the exiting gas flow. Without the monolith insert, the plasma flows through the discharge tube with a clear circular cross-sectional area of 79 mm2. However the monolith cross section consists of a honeycomb-like pattern of square- shaped holes from which gas must travel through. Each monolith has a diameter just under 10 mm to fit snugly into the discharge tube, resulting in approximately 30 holes per cross section, each with an inner area of 1.4 mm2. Thus with the presence of the monolith, the total gas-flow cross section becomes 45 mm2, a 43% reduction. From conservation of mass shown in Equation 6.7 with the substitution ρ = P/RT using the Ideal Gas Law, there must be a change in particle velocity, pressure, or temperature when the cross-sectional area changes. Here m ̇ is mass flow rate, ρ is gas density, v is 139PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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