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2. HYDROGEN RADICAL ASSISTED METHANATION Table 2.3: Reactions occurring only in the arc. Name Reaction Rate coefficient A1 Ar+e−→Ar+ +e+e f(Te) A2 H2+e−→H+H+e f(Te) 2.4. DISCUSSION A3 0.20 0.16 0.12 0.08 0.04 0.00 H + H(wall) −→ H2rv Depends on surface Ar+ H 0.0 0.2 0.4 0.6 0.8 1.0 Figure 2.6: Calculated mixing ratios of Ar+ and H as a function of Φ (see equation 2.1) are charge transfer and dissociative recombination. In the ion-driven regime, these two occur in a sequence: CT followed by DR. Ar+ +AB−→Ar+AB+ (CT) AB+ + e −→ A + B (DR) where AB is a molecular species which can dissociate into A and B and CT refers to charge transfer reaction and DR refers to dissociative recombination reaction. Although there are two charge transfer reactions possible between H2 and Ar+ ions only reaction C3 (table 2.4) is very likely at low electron temperatures of EPJ [102]. Using concentrations of H radicals and Ar+ ions (10% of input H2 and Ar respect- ively) produced by the arc as the starting point and considering the CT and DR reactions 28 Mixing ratioPDF Image | Understanding CO2 containing non-equilibrium plasmas
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