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Density of asymmetric mode (001) (1014 cm−3) 1 0.8 0.6 0.4 0.2 0 60 80 5 4 3 2 1 100 120 140 Time (μs) Density of asymmetric mode (002) (1014 cm−3) a) 1 0.8 0.6 0.4 0.2 0 60 80 12 10 8 6 4 2 100 120 Time (μs) 140 Figure 5.8: Spatiotemporal distribution of asymmetric modes CO2(v31) and (002) for the same conditions used in Fig 5.7. Voltage is switched off after 10 cycles at t0 = 77 μ s marked with pink line. See the text for explanation. however, that the initial conditions the densities considered are very low so as to match the initial conditions of the calculations done in chapter 4. These trends can be explained considering the production and loss rates of each spe- cies. Let us assume that n1 , n2 , ne and n0 are the densities of CO2 (v31 ), CO2 (v32 ), electrons and CO2(v0) respectively. Then the rate of change of n1 can be written as dn1 = −kV T n1n0 −k1n1n1 −kV en1ne +keV n0ne +kV T2n2n0 +kV e2n2ne (5.11) dt where k1, keV and keV are the rate coefficient of VV transfer (VV2), electronic ex- citation (E8) and electronic de-excitation (E9) reactions, keV 2 is the rate coefficient of electron impact de-excitation from CO2(v32) (E35). kV T includes two VT relaxation reactions to the ground state: VT7 to CO2(v4) and VT6 to CO2(v1); kV T2 is VT relaxa- 136 5.9. RESULTS & DISCUSSION Position (mm) Position (mm) b)PDF Image | Understanding CO2 containing non-equilibrium plasmas
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