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Molecules 2020, 25, 5572 9 of 26 Figure 8. (a) Even- and odd-numbered aliphatic chains in the α phase. The absence of tilting in respect to the end-group plane in this polymorph generates no change in the long spacings (d) between even- and odd-numbered molecules. (b) Even- and odd-numbered aliphatic chains in β’ or β phases, where tilting occurs. Here, the tilting of the plane causes an enlargement in the long spacings of odd-numbered chains. Images reproduced from Malkin [24]. Figure 9. Enthalpies of fusion [J/g] collected in literature of the α (black, round), β’ (red, diamond) and β (blue, triangle) phases of saturated symmetrical triglycerides plotted against the carbon number of the precursor fatty acids (between 8 and 24). Similarly to what observed for the melting points, an alternation between odd- and even-numbered triglycerides can be noticed for all polymorphic phases. A clear alternation between the properties of odd-even numbered chains is reflected in the enthalpies of fusion; those of odd-numbered chains are consistently lower than their even-numbered counterparts. This also appears for the β polymorph, while due to lack of additional data it is unclearPDF Image | Triglycerides as Novel Phase-Change Materials
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