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Fu et al. In situ Catalytic Transformation SCHEME 4 | CO2 capture and transformation to oxazolidinones. SCHEME 5 | Synthesis of β-oxopropylcarbamates from propargylic alcohols and ammonium carbamates. 10% Na2 CO3 /Al2 O3 have a methanation capacity of 0.91 and 1.05 g-mol/kg DFM, respectively. Similarly, A. Urakawa group develops the catalyst consisting of earth-abundant chemical elements (FeCrCu/K/MgO–Al2 O3 ), which can trap CO2 from fuel gas in the form of surface carbonates and subsequently hydrogenated the adsorbed CO2 to CO (Bobadilla et al., 2016). Accordingly, these DFMs are identified as promising candidates for CO2 capture and direct utilizations. Hydrogenation of captured CO2 to energy chemicals can facilitate turning hydrogen gas to liquid fuel as well as realize carbon cycling. Albeit the hydrogenation of captured CO2 has been extensively investigated and various capture reagents and catalysts have been developed, the identification of CO2 activation forms is still controversial. For example, the CO2 capture products alkyl carbonate ammonium salts are considered as the activated CO2 species (Li et al., 2013, 2014; Su et al., Frontiers in Chemistry | www.frontiersin.org 6 July 2019 | Volume 7 | Article 525PDF Image | CO2 Capture and in situ Catalytic Transformation
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