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Materials 2021, 14, 1786 Materials 2021, 14, 1786 7 of 19 7 of 20 bonds involving the adjacent layers and the crystallization water molecules, ultimately leading to a three-dimensional (3D) supramolecular framework (H-bonds not shown). FFiigurree22..SSttrrucctturrallffeattures of the crystal structure of TbCP1:: (a) two-diimenssiionaall((22D))ssuupprraamoole-c- lecular network extended in the [001] direction of the unit cell, with the O−H···O hydrogen bonds ular network extended in the [001] direction of the unit cell, with the O–H···O hydrogen bonds drawn drawn as light-blue dashed lines and the π-π stacking interactions represented as a grey shadow as light-blue dashed lines and the π-π stacking interactions represented as a grey shadow (one of the (one of the coordination chains are shown in yellow color). (b) Extended packing arrangement coordination chains are shown in yellow color). (b) Extended packing arrangement viewed in the viewed in the [100] direction of the unit cell with the crystallization water molecules occupying the [100] direction of the unit cell with the crystallization water molecules occupying the cavities (these cavities (these water molecules are drawn in a space fill model and orange/yellow color scheme). water molecules are drawn in a space fill model and orange/yellow color scheme).PDF Image | Green Chemistry with Supercritical CO2 and Enzymes
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