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10-year goals: • New FTS catalysts for selective and stable operation in CO2/H2 feeds, e.g. stabilization of iron carbide catalysts at high CO2/H2O partial pressures • Direct synthesis of dimethyl ether from CO2/H2 feeds • Predictive design of CO2 hydrogenation catalysts and their transient behavior • Evolution from pilot plants to full scale for methanation and methanol synthesis • Demonstration of an industrial RWGS process with downstream CO conversion to methanol • Piloting new CO2 converting processes for materials and chemicals • New dedicated catalyst composites for coupled reactions and chemical looping reactors 3.5 Conclusion The preceding discussion has highlighted a range of excellent opportunities for the production of chemicals, fuels, and materials derived from CO2 and sustainable hydrogen. Today, several of the presented technologies are within reach, with several having already been developed into demonstrator projects. However, further research on the synthesis of new catalysts, which is coupled to developments in state-of-the-art synthesis, theory, and characterization, and on reaction and reactor engineering concepts, is urgently needed. References 1G. A. Olah, “Beyond oil and gas: the methanol economy”, Angewandte Chemie International Edition, 44, 2636–2639 (2005). 2Methanol fuel from CO2, http://www.mefCO2.eu, Accessed: 2019-07-03. 3M. Bowker, “Methanol synthesis from CO2 hydrogenation”, ChemCatChem, 10.1002/cctc.201900401. 4M. Behrens, F. Studt, I. Kasatkin, S. Ku ̈hl, M. H ̈avecker, F. Abild-Pedersen, S. Zander, F. Girgsdies, P. Kurr, B.-L. Kniep, M. Tovar, R. W. Fischer, J. K. Nørskov, and R. Schl ̈ogl, “The Active Site of Methanol Synthesis over Cu/ZnO/Al2O3 Industrial Catalysts”, Science, 336, 893–897 (2012). 5R. Van Den Berg, G. Prieto, G. Korpershoek, L. I. Van Der Wal, A. J. Van Bunningen, S. Lægsgaard- Jørgensen, P. E. De Jongh, and K. P. De Jong, “Structure sensitivity of Cu and CuZn catalysts relevant to industrial methanol synthesis”, Nature Communications, 7, 13057 (2016). 6S. Kuld, M. Thorhauge, H. Falsig, C. F. Elkjær, S. Helveg, I. Chorkendorff, and J. Sehested, “Quantifying the promotion of Cu catalysts by ZnO for methanol synthesis”, Science, 352, 969–974 (2016). 36PDF Image | sustainable production of fuels and chemicals
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