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Jen Wade — for teaching me how to assemble high-temperature experimental set- ups and helping me begin experiments, and for the valuable discussions and productive times. Tuncel Yegulalp — for introducing me to data analysis and modeling techniques. The first/second generation Lackner group — for being such an enjoyable group full of ideas and enthusiasm to embark on the fascinating and wild ride of PhD studies under Klaus. I hope that we keep in touch throughout our new careers! Søren Koch, Jens Borchsenius, and Ebtisam Abdellahi — for helping me set up and improve lab experiments. Søren Koch and Karin Vels Hansen — for having built an excellent automated control and data acquisition system the usefulness of which cannot be overstated. Nikos Bonanos, Tânia Ramos, Kent Kammer Hansen, and Karin Vels Hansen — for many valuable discussions about impedance spectroscopy and materials. Søren Højgaard Jensen, Anne Hauch, Peter Blennow, Jens Høgh, and Karin Vels Hansen for each writing excellent, well-documented and inspirational dissertations that gave me a basis for parts of my experimental work, and for discussing your work with me. Jason Wang, a great office-mate and friend. The rest of my fellow students and colleagues at Columbia and Risø. You are too many to mention but have all contributed. The enjoyable discussions and working environments were greatly appreciated. Uncle Pat for being genuine and supportive, wish you were here to see the outcome. Special thanks to my friends and family for support and understanding while I tended to almost completely disappear and become a hermit for well over a year. Of course to my Kalee for love, patience, and support, and for taking a leap and joining the cross-Atlantic journey to Denmark. Without you this truly would not have been possible. — I would also like to thank the authors of the free and open-source Python libraries NumPy and Matplotlib, which made the data analysis and plotting enjoyable. Financial support from the American Chemical Society Petroleum Research Fund, from the Lenfest Center for Sustainable Energy, and from the Programme Commission on Sustainable Energy and Environment, The Danish Council for Strategic Research, via the SERC project, is gratefully acknowledged. xvPDF Image | Electrolysis of CO2 and H2O
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