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be well-chosen. In the following subchapter the advantages of implementing zeolite membranes in catalytic reactions are reviewed for spatial decoupled processes before we proceed with arrays of membranes and catalysts in close contact with each other in the following main chapters. 2.3.Zeolit2e.3M.ZemeoblirtaenMeeSmebprarnaetiSoenpaSrpataitoinalSlypaDtieaclloyuDpleecdoufprloemdftrhoemCthaetaClaytaiclyUticniUtnit Zeolite membrane modules could be applied apart from the reaction zone as Zeolite membrane modules could be applied apart from the reaction zone as alternatives to the alternatives to the complex conventional separation processes. Figure 2 reveals two complex conventional separation processes. Figure 2 reveals two application possibilities of zeolite application possibilities of zeolite membranes where the separation process is either membranes where the separation process is either for (i) feed treatment (Figure 2A) or (ii) product for (i) feed treatment (Figure 2A) or (ii) product treatment (Figure 2B) with optional treatmentr(eFtiegnutraete2sBtr)ewamithreocpytciolen.aTlhretecuntraretentstcrheampterrecbyricelfle.yTdhiesccuusrsresnotnclhyapextearmbprilefslywdhiesrceussesonly examples where the catalytic process is spatially decoupled from the membrane unit. the catalytic process is spatially decoupled from the membrane unit. Figure 2. Schematic drawing of different set-ups of zeolite membranes apart from Figure 2. Schematic drawing of different set-ups of zeolite membranes apart from the the reaction zone; (A) feed treatment; and (B) product treatment with optional reaction zone; (A) feed treatment; and (B) product treatment with optional retentate recycle. Starting with the feed treatment configuration, the membrane module could be used to adjust the feed retentate recycle. Starting with the feed treatment configuration, the membrane module could stream in order to intensify processes. Beside polymer membranes [117], MFI zeolite membranes can be used to adjust the feed stream in order to intensify processes. Beside polymer membranes [117], MFI zeolite membranes can be applied for the conditioning of natural gas [118]. Simplified natural gas model mixtures comprising methane and n-butane were separated with high efficiency under permeate vacuum [115]. Well-pronounced loading gradients across the membrane, decreased coverages of the adsorbed n-butane molecules at the permeate side as well as decreased diffusion resistances were registered. The resulting permeate streams, highly enriched with n-butane, were converted with steam at low (450 ◦C) and high (750 ◦C) temperatures over 1 wt. % Rh/γ-Al2O3 for syngas production [119]. The positive influence of the membrane upstream on the steam reforming was demonstrated. For example, at a 10PDF Image | Zeolite Catalysis
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