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43 Reactor Reaction Type Feed Operating Conditions Core-Shell Catalyst Xmixed (%) Smixed (%) Ymixed (%) XMR. (%) SMR. (%) YMR. (%) References Direct synthesis of PLMR middle i-paraffins catalytic hydrogen and carbon monoxide 300 ◦C p = 1 MPa H2/CO = 1 H-ZSM-5 coated on Fe/SBA-15 XCO = 63.9 SCO2 = 43.8 SCH4 = 19.2 Sn =56 XCO = 57.6 SCO2 = 37.3 SCH4 = 15.3 Sn =36.7 [244] Direct synthesis of PMLR i-paraffins catalytic carbon monoxide, hydrogen 280 ◦C p = 1 MPa H2/CO = 1 SCO2 = 29.9 SCH4 = 7 Si = 12.9 SCO2 = 33.8 SCH4 = 14.9 Si = 29.8 [260] Dimethyl ether PLMR direct synthesis catalytic hydrogen, carbon monoxide, carbon dioxide and argon 523 K p = 5.0 MPa H-ZSM-5 coated on Cu/ZnO/Al2O3 XCO = 58.07 SMeOH = 57.29 SDME = 40.51 XCO = 30.4 SMeOH = 21.43 SDME = 78.57 [261] Dimethyl ether PLMR direct synthesis catalytic hydrogen, carbon monoxide, carbon dioxide and argon 573-623 K p = 5.0 MPa Double layer H-ZSM-5/Silicalite-1 membrane coated on Cr/ZnO core catalyst Double layer H-ZSM-5/Silicalite-1 membrane coated on Pd/SiO2 core catalyst XCO = 45.16 SMeOH = 12.12 SDME = 0.47 XCO = 9.53 SMeOH = 21.23 SDME = 50.84 [262] Dimethyl ether PLMR direct synthesis catalytic 523 K p = 5.0 MPa SCH4 = 16.8 SMeOH = 4.76 SDME = 68.70 [263] Dimethyl ether PLMR direct synthesis catalytic 350 ◦C p = 5 MPa SCH4 = 3.7 SMeOH = 71.7 SDME = 16.5 SCH4 = 4.7 SMeOH = 52.2 SDME = 37.0 [243] hydrogen, carbon monoxide, carbon dioxide, argon XCO = 12.84 SCH4 = 1.47 SMeOH = 16.51 SDME = 48.40 XCO = 9.48 hydrogen, carbon monoxide, carbon dioxide, argon SAPO-46 zeolite shell encapsulated Cr/ZnO catalyst XCO = 4.7 XCO = 6.9 Table 2. Cont. Silicalite-1 and H-ZSM-5 coated on Fe/SiO2 dual-membrane coated catalyst Si = 33.9 XCO = 60 Si = 46.5 XCO = 54.8PDF Image | Zeolite Catalysis
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