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Catalysts 2015, 5 2202 Figure 13. Scheme of the synthesis procedure of HMOR/FI capsule catalysts Figure 13. Scheme of the synthesis procedure of HMOR/FI capsule catalysts (FI = Fused (FI = Fused Iron) without template and product distributions during Iron) without template and product distributions during Fischer-Tropsch synthesis (operating Fischer-Tropsch synthesis (operating conditions: H2/CO = 1/1, 1.0 MPa, 300 ◦C, conditions: H2/CO = 1/1, 1.0 MPa, 300 °C, 10 gFI·h−1·mol−1) obtained using (a) pure FI; 10 gFI·h−1·mol−1) obtained using (a) pure FI; (b) Silicalite-1/FI; (c) HMOR + FI; (b) Silicalite-1/FI; (c) HMOR + FI; and (d) HMOR/FI. Reprinted with permission from [281]. and (d) HMOR/FI. Reprinted with permission from [281]. Copyright (2013) Copyright (2013) John Wiley and Sons. John Wiley and Sons. Very recently, Jin et al. [260] developed a novel dual-membrane coating Fe/SiO2 catalyst core with Another research incentive comes from the request to design appropriate silicalite-1 and H-ZSM-5 zeolite membranes following a previously reported synthesis procedure for catalysts for the direct production of dimethyl ether (DME) being considered as double-shell capsule catalyst [262]. The silicalite-1 synthesized under close-to-neutral condition was a basic feedstock and a clean fuel [288]. Beside the dehydration of methanol acting as catalyst protective membrane for the core with high iron loading, whereas the (produced from syngas) to DME, a more desired and thermodynamically favorable H-ZSM-5 was the active membrane for the synthesis of i-paraffins. The authors stressed that alternative is the direct conversion of syngas to DME over hybrid catalysts [289–293]. attempts to coat H-ZSM-5 directly over high iron loading Fe/SiO2 core failed due to the strong alkaline conditions required for its synthesis. The i-paraffin selectivity of 29.8% being higher 53 than that of Fe/SiO2 catalyst (12.9%) and the physical mixture (16.6%) was attributed to the combinationPDF Image | Zeolite Catalysis
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