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Conclusion Solid sorbents offer a potential solution to the carbon capture problem, as they are extremely promising materials for efficient, selective sorption of CO2 and other relevant gases. Although the sorbent materials developed to date are usable, they need further significant improvements to become practical. Incremental modification of the current materials is unlikely to provide a solution. Instead, a whole new generation of materials is needed whose structures and dynamics can be precisely controlled across multiple length scales, from the atomic level to macroscale. The development of such advanced structures will require significant advances in materials modeling, synthesis, and characterization, as well as a detailed understanding of the structure–properties relationships in materials. References 1. M. Nakashima, S. Shimada, M. Inagaki, and T. A. Centeno, “On the adsorption of CO2 by molecular-sieve carbons—Volumetric and gravimetric studies,” Carbon 33(9), 1301–1306 (1995). 2. R. V. Siriwardane, M. S. Shen, E. P. Fisher, and J. A. Poston “Adsorption of CO2 on molecular sieves and activated carbon,” Energy and Fuels 15(2) 279–284, March–April (2001). 3. C. Pevida, M. G. Plaza, B. Arias, J. Fermoso, F. Rubiera, and J. J. Pis, “Surface modification of activated carbons for CO2 capture,” Applied Surface Science 254(22) 7165–7172 (September 15, 2008). 4. M. G. Plaza, C. Pevida, A. Arenillas, F. Rubiera, and J. J. Pis, “CO2 capture by adsorption with nitrogen enriched carbons,” Fuel 86(14), 2204–2212 (September 2007). 5. J. C. Hicks, J. H. Drese, D. J. Fauth, M. L. Gray, G. G. Qi, and C. W. Jones, “Designing adsorbents for CO2 capture from flue gas-hyperbranched aminosilicas capable of capturing CO2 reversibly,” Journal of the American Chemical Society 130(10), 2902–2903 (March 12, 2008). 6. A. L. Chaffee, G. P. Knowles, Z. Liang, J. Zhany, P. Xiao, and P. A. Webley, “CO2 capture by adsorption: Materials and process development,” International Journal of Greenhouse Gas Control 1(10), 11–18 (April 2007). 7. R. Serna-Guerrero, E. Da’na, and A. Sayari, “New insights into the interactions of CO2 with amine-functionalized silica,” Industrial and Engineering Chemistry Research 47(23), 9406–9412 (November 5, 2008). 8. X. C. Xu, C. S. Song, B. G. Miller, and A. W. Scaroni, “Influence of moisture on CO2 separation from gas mixture by a nanoporous adsorbent based on polyethylenimine- modified molecular sieve MCM-41,” Industrial and Engineering Chemistry Research 44(21), 8113–8119 (October 12, 2005). 9. O. Yaghi, M. O’Keeffe, N. W. Ockwig, H. K. Chae, M. Eddaoudi, and J. Kim, “Reticular synthesis and the design of new materials,” Nature L 423, 705–714 (2003). 10. J.-R. Li, R. J. Kuppler, and H.-C. Zhou, “Selective gas adsorption and separation in metal–organic frameworks,” Chem. Soc. Rev. 38, 1477–1504 (2009). 11. B. Wang, A. P. Côté, H. Furukawa, M. O’Keeffe, and O. M. Yaghi, “Colossal cages in zeolitic imidazolate frameworks as selective carbon dioxide reservoirs,” Nature 453, 207–211 (2008). 23PDF Image | 2020 Carbon Capture
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